The Gyroscope is found in a treasure sphere at the Crash Site in the north Wildlands. You will need to have the Chocobo healed enough to glide (so completion of Chapter 3-2) to reach it.
The Moogle Dust is found in the Moogle Village (in Jagd Woods in the Wildlands) on a path leading to the centre of the village. You can’t miss it really. Be aware that the village can only be entered between 19:00 - 07:00.
This item can only be collected between 11:00 - 16:00 every day and is found by facing the steps to the upper reaches of the Industrial Area (in Yusnaan) and then looking left.
See the main quest guide for the Temple Ruins to find it. It is found in the Scorched Earth Upper Level part of the Temple Ruins close to Nolan who gives you the “What Rough Beast Slouches” quest.
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